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  • May
    30

    EES Seminar- Plasmon- Mediated Advanced Reduction Processes for Contaminant Degradation: PFAS and Nitrate- Haklae Lee

    McCormick - Civil and Environmental Engineering (CEE)

    2:00 PM A230, Technological Institute

    EVENT DETAILS

    Abstract

    The use of nanomaterials has become a rapidly growing approach for advanced water treatment technologies, but the continued emergence of highly oxidation-resistant micropollutants, such as per- and polyfluoroalkyl substances (PFAS), calls for transformative strategies that move beyond recent oxidation-based remediation practices. Alternative reduction-based approaches utilizing aqueous electrons (eaq−, Eo = −2.9 V)—one of the most reactive nucleophilic species—are emerging as a promising solution for efficient PFAS breakdown. Herein, we leverage nanoconfinement engineering to enable a new water treatment approach—plasmon-mediated advanced reduction processes (PARPs)—for efficient, chemical-free PFAS destruction at room temperature. We first present novel nanoreactor designs that engineer the ‘nanoconfinement effect’, i.e. unique aggregation-induced interparticle interactions that are inaccessible by typical unconfined, bulk-phase nanomaterials. We demonstrate that the precisely controlled nanoconfinement of plasmonic nanoparticles can generate highly reactive reducing species under UV irradiation, capable of breaking even the strong C–F bonds in PFAS. The nanoreactor we developed achieved 81.5% mineralization of perfluorooctanoic acid (PFOA) after 24 hours of UV irradiation in pure water at room temperature, compared to only 16.6% mineralization by UV photolysis. Further reaction monitoring under various conditions and multimodal NMR-guided investigation were conducted to elucidate PFAS degradation mechanisms and pathways. We further explored the potential of PARPs for the chemical-free remediation of nitrate, a prevalent oxyanion pollutant that is resistant to conventional oxidation-based treatments. Our findings highlight the transformative promise of nanoconfinement engineering to catalyze innovation in environmental nanotechnology and extend the frontier of advanced reduction processes for water treatment.

    Bio- Haklae Lee is a PhD student in the Environmental Engineering & Science program and a member of the Gray Lab in the Department of Civil and Environmental Engineering at Northwestern University. He holds a B.S. and M.S. in Environmental Engineering from Pusan National University in South Korea. His work focuses on the design and engineering of nano-sized reactors for efficient and more sustainable remediation of emerging contaminants from wastewater. He uses mesoporous silica to spatially confine various metal nanoparticles within multi-layered nanoreactors, enabling unique features such as multifunctional compartments and nanoconfinement effects for previously unexplored environmental applications.

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    TIME Friday, May 30, 2025 at 2:00 PM - 3:00 PM

    LOCATION A230, Technological Institute    map it

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    CONTACT Andrew Liguori    andrew.liguori@northwestern.edu EMAIL

    CALENDAR McCormick - Civil and Environmental Engineering (CEE)

  • Sep
    8

    Welcome & Breakfast for New McCormick PhD Students

    McCormick School of Engineering and Applied Science

    9:00 AM LR2 & Tech East Plaza, Technological Institute

    EVENT DETAILS

    TIME Monday, September 8, 2025 at 9:00 AM - 10:00 AM

    LOCATION LR2 & Tech East Plaza, Technological Institute    map it

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    CONTACT Andi Joppie    andi.joppie@northwestern.edu EMAIL

    CALENDAR McCormick School of Engineering and Applied Science

  • Sep
    12

    New Undergraduate Fall 2025 Registration

    University Academic Calendar

    All Day

    EVENT DETAILS

    TIME Friday, September 12, 2025

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    CONTACT Office of the Registrar    nu-registrar@northwestern.edu EMAIL

    CALENDAR University Academic Calendar

  • Sep
    15

    Welcome & Luncheon for New Full-time Graduate Students

    McCormick School of Engineering and Applied Science

    11:00 AM Ryan Auditorium & Tech East Plaza, Technological Institute

    EVENT DETAILS

    TIME Monday, September 15, 2025 at 11:00 AM - 12:30 PM

    LOCATION Ryan Auditorium & Tech East Plaza, Technological Institute    map it

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    CONTACT Andi Joppie    andi.joppie@northwestern.edu EMAIL

    CALENDAR McCormick School of Engineering and Applied Science

  • Sep
    16

    Fall Classes Begin. Change of Registration (Drop/Add) Late registration for returning students begins

    University Academic Calendar

    All Day

    EVENT DETAILS

    TIME Tuesday, September 16, 2025

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    CONTACT Office of the Registrar    nu-registrar@northwestern.edu EMAIL

    CALENDAR University Academic Calendar

  • Sep
    24

    SPREE Seminar

    McCormick - Civil and Environmental Engineering (CEE)

    11:00 AM A230, Technological Institute

    EVENT DETAILS

    TIME Wednesday, September 24, 2025 at 11:00 AM - 12:00 PM

    LOCATION A230, Technological Institute    map it

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    CONTACT Andrew Liguori    andrew.liguori@northwestern.edu EMAIL

    CALENDAR McCormick - Civil and Environmental Engineering (CEE)

  • Sep
    26

    EES Seminar

    McCormick - Civil and Environmental Engineering (CEE)

    2:00 PM A230, Technological Institute

    EVENT DETAILS

    TIME Friday, September 26, 2025 at 2:00 PM - 3:00 PM

    LOCATION A230, Technological Institute    map it

    ADD TO CALENDAR

    CONTACT Andrew Liguori    andrew.liguori@northwestern.edu EMAIL

    CALENDAR McCormick - Civil and Environmental Engineering (CEE)

  • Sep
    29

    AED-MPM Seminar

    McCormick - Civil and Environmental Engineering (CEE)

    11:00 AM A230, Technological Institute

    EVENT DETAILS

    TIME Monday, September 29, 2025 at 11:00 AM - 12:00 PM

    LOCATION A230, Technological Institute    map it

    ADD TO CALENDAR

    CONTACT Andrew Liguori    andrew.liguori@northwestern.edu EMAIL

    CALENDAR McCormick - Civil and Environmental Engineering (CEE)

  • Oct
    1

    SPREE Seminar

    McCormick - Civil and Environmental Engineering (CEE)

    11:00 AM A230, Technological Institute

    EVENT DETAILS

    TIME Wednesday, October 1, 2025 at 11:00 AM - 12:00 PM

    LOCATION A230, Technological Institute    map it

    ADD TO CALENDAR

    CONTACT Andrew Liguori    andrew.liguori@northwestern.edu EMAIL

    CALENDAR McCormick - Civil and Environmental Engineering (CEE)